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Robust optical polarization of nuclear spin baths using Hamiltonian engineering of nitrogen-vacancy center quantum dynamics

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peer-reviewed

Erstveröffentlichung
2018-08-31
Authors
Schwartz, Ilai
Scheuer, Jochen
Tratzmiller, Benedikt
Müller, Samuel
Chen, Qiong
et al.
Wissenschaftlicher Artikel


Published in
Science Advances ; 4 (2018), 8. - Art.-Nr. eaat8978. - eISSN 2375-2548
Link to original publication
https://dx.doi.org/10.1126/sciadv.aat8978
Faculties
Fakultät für Naturwissenschaften
Institutions
Institut für Theoretische Physik
Institut für Quantenoptik
External cooperations
NVision Imaging Technologies Gmbh
Document version
published version (publisher's PDF)
Abstract
Dynamic nuclear polarization (DNP) is an important technique that uses polarization transfer from electron to nuclear spins to achieve nuclear hyperpolarization. Combining efficient DNP with optically polarized nitrogen-vacancy (NV) centers offers promising opportunities for novel technological applications, including nanoscale nuclear magnetic resonance spectroscopy of liquids, hyperpolarized nanodiamonds as magnetic resonance imaging contrast agents, and the initialization of nuclear spin–based diamond quantumsimulators. However, none of the current realizations of polarization transfer are simultaneously robust and sufficiently efficient, making the realization of the applications extremely challenging. We introduce the concept of systematically designing polarization sequences by Hamiltonian engineering, resulting in polarization sequences that are robust and fast. We theoretically derive sequences and experimentally demonstrate that they are capable of efficient polarization transfer from optically polarized NV centers in diamond to the surrounding 13C nuclear spin bath even in the presence of control errors,making the abovementioned novel applications possible.
EU Project uulm
BIOQ / Diamond Quantum Devices and Biology / EC / FP7 / 319130
DFG Project THU
SFB 1279 / Nutzung des menschlichen Peptidoms für die Entwicklung neuer antimikrobieller und anti-Krebs Therapeutika / DFG / 316249678
Publication funding
Gefördert vom Ministerium für Wissenschaft, Forschung und Kunst Baden-Württemberg
Is supplemented by
http://advances.sciencemag.org/content/suppl/2018/08/27/4.8.eaat8978.DC1
Subject headings
[GND]: NMR-Spektroskopie | Hamiltonsches System
[LCSH]: Optically stimulated luminescence | Nuclear magnetic resonance spectroscopy | Hamiltonian systems
[DDC subject group]: DDC 530 / Physics | DDC 620 / Engineering & allied operations
License
CC-BY-NC International 4.0
https://creativecommons.org/licenses/by-nc/4.0/

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DOI & citation

Please use this identifier to cite or link to this item: http://dx.doi.org/10.18725/OPARU-36761

Schwartz, Ilai et al. (2021): Robust optical polarization of nuclear spin baths using Hamiltonian engineering of nitrogen-vacancy center quantum dynamics. Open Access Repositorium der Universität Ulm und Technischen Hochschule Ulm. http://dx.doi.org/10.18725/OPARU-36761
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